Research Progress on Preparation of Two-dimensional h-BN and Application in Anti-corrosion Coatings

FENG Xuelian; LI Guihua; LIU Xiaoyan; GAO Yuanming; BAI Yu; MA Wen

doi:10.16490/j.cnki.issn.1001-3660.2025.22.002

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Surface Technology ›› 2025, Vol. 54 ›› Issue (22) : 16-30. DOI: 10.16490/j.cnki.issn.1001-3660.2025.22.002

Research Review

Research Progress on Preparation of Two-dimensional h-BN and Application in Anti-corrosion Coatings

FENG Xuelian, LI Guihua^*, LIU Xiaoyan, GAO Yuanming, BAI Yu, MA Wen

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Abstract

Hexagonal boron nitride, as a typical two-dimensional material, demonstrates significant application potential in anti-corrosion coatings by virtue of its excellent high-temperature stability, chemical inertness, and electrical insulation. Research shows monolayer or multilayer h-BN in coatings generate "labyrinth effect", providing superior corrosion protection than multilayer h-BN. However, the partial ionic bonding characteristics between boron and nitrogen atoms within h-BN interlayers make it difficult to exfoliate h-BN into monolayer or multilayer nanosheets. To solve this problem, researchers are developing efficient preparation methods for h-BN nanosheets, which is particularly crucial for the practical application of h-BN practical applications in corrosion prevention.
This paper systematically reviews the research progress on preparation of two-dimensional hexagonal boron nitride (h-BN) and its application in organic anti-corrosion coatings. The content encompasses multiple aspects, including the crystal structure, material properties, preparation methods, and applications in organic anti-corrosion coatings of h-BN.
Firstly, the crystal structure characteristics and key material properties of h-BN are briefly described. As one of the most common crystalline forms of boron nitride, h-BN features a layered structure similar to graphite. Within each layer, boron (B) and nitrogen (N) atoms are alternately arranged in a 1∶1 ratio to form a honeycomb-like structure, while the adjacent layers are connected by van der Waals forces. Compared with graphite, h-BN not only exhibits comparable mechanical strength and thermal properties but also possesses additional superior characteristics, such as being electrically insulating and having a chemically inert surface.
Secondly, the methods for preparing h-BN nanosheets are discussed in detail, which are primarily categorized into two major classes: one is the "top-down" approach (such as mechanical exfoliation, liquid-phase exfoliation, intercalation methods, etc.), and the other is the "bottom-up" approach (such as chemical vapor deposition, physical vapor deposition, etc.). At the same time, the prominent advantages and disadvantages of various preparation methods in terms of yield, cost control, uniformity, and feasibility of large-scale production are compared in detail. For example, the "top-down" approachs have a simple operation process but uneven product quality, while the "bottom-up" approachs can achieve precise structural control, but are limited by equipment complexity and cost-effectiveness.
Furthermore, this article also discusses in detail the application research progress of h-BN nanosheets in organic anti-corrosion coatings, focusing on three typical polymer coating systems: epoxy resin, polyurethane, and acrylic resin. By comparing and analyzing the corrosion resistance evolution of the coating system before and after modification with h-BN nanosheets, the enhancement mechanisms are deeply elucidated, including key mechanisms such as physical barrier effects, prolonged diffusion path of corrosive medium, and interfacial bonding reinforcement. These key mechanisms lay a solid foundation for the application of h-BN nanosheets in organic anti-corrosion coatings.
Finally, based on the systematic summary of the existing research progress of h-BN nanosheets, this paper briefly analyzes the technical bottlenecks currently faced by h-BN nanosheets from the aspects such as preparation process, dispersion effect, and protective performance. And the future development direction is predicted, providing a valuable reference for expanding the research and application of h-BN in the anti-corrosion field.

Key words

hexagonal boron nitride / preparation method / organic anti-corrosion coating / epoxy resin / polyurethane / acrylic resin

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FENG Xuelian, LI Guihua, LIU Xiaoyan, GAO Yuanming, BAI Yu, MA Wen. Research Progress on Preparation of Two-dimensional h-BN and Application in Anti-corrosion Coatings[J]. Surface Technology. 2025, 54(22): 16-30 https://doi.org/10.16490/j.cnki.issn.1001-3660.2025.22.002

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Funding

Natural Science Foundation Project of Inner Mongolia Autonomous Region (2024QN05003); Science and Technology Program Project of Inner Mongolia Autonomous Region (2025KYPT0027); First-Class Discipline Scientific Research Special Project of Inner Mongolia Autonomous Region (YLXKZX-NGD-040)